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A8=uU>$.R̆K{2!Nqd!$ ZZaJR@Êg&樬ꝺxRarJ%+)Fj܁d J8Th1pLF5 ME)g."JH)-F|W(m']N-N#$yB_л|nnNr̪YyaΎ2p6Q%0xΈ72Sj%"e@Mmz3!Y]<\,dܚ@iͅY']nF Rц7fGeF-.PI_zH푉SUy Oije; ˔gIl ӊKS;FYQZ@|$)uG|,mA1 B*f$Y|* #jk )@?͌.oR: ڼ96@5FIꐿ!`cǔOo mΗ젢RlcVJc&1I֕U!e`1O$\3R_6|jYZlԮ $b_am{;$j0%7Cq:R^!Y>& W ΄k ?Ǣ1'K?'9O0v$uMg\tf"Ls-$s1b.xH8` LcNH5xJj-QS;}z`{^Р/џYд4(,ۉXLGq%=-nV6\lToxׇYt?ȒtA"(1^ԡ`":s(d%yMB gzap9$gm 5'ew3F`Z=gOM5pOڌ2rsf4ZWLN]L@\#ӿ|#Il਷^SUj+ۑų*·g.p1Z`4"[pYsF[6BiWt (V-Bzj~{,"۝~ka A6J25wxJ̆P7)qP*wpQiø7N9cSyb?n0%)X6 yTEq2ouЉu%}#ŝ Gqܦti{DƥlǞ.њؐ^H#Bt)kƿ? endstream endobj 508 0 obj <> endobj 509 0 obj <> endobj 510 0 obj <> endobj 511 0 obj <> endobj 512 0 obj <> endobj 513 0 obj <> endobj 514 0 obj <> endobj 515 0 obj <> endobj 516 0 obj <> endobj 517 0 obj <> endobj 518 0 obj <> endobj 519 0 obj <> endobj 1 0 obj <> endobj 2 0 obj [3 0 R 4 0 R 5 0 R 6 0 R 7 0 R 8 0 R 9 0 R 10 0 R 11 0 R] endobj 3 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 1 | Morphology and elemental distribution in bare LCO and TMA-LCO. a,b,\ Scanning electron microscopy \(SEM\) images of bare LCO \(a\) and TMA-LCO \(b\). Scale bars: 20 m. c, Cross-sectional TEM i\ mage of TMA-LCO. Scale bar: 2 m. d:2539)/F 4/H/N/Rect[58.7371 170.706 73.8588 158.16]/Subtype/Link/Type/Annot>> endobj 4 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 1 | Morphology and elemental distribution in bare LCO and TMA-LCO. a,b\ , Scanning electron microscopy \(SEM\) images of bare LCO \(a\) and TMA-LCO \(b\). Scale bars: 20 m. c, Cross-sectional TEM \ image of TMA-LCO. Scale bar: 2 m. :2540)/F 4/H/N/Rect[195.086 118.206 204.461 105.66]/Subtype/Link/Type/Annot>> endobj 5 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 1 | Morphology and elemental distribution in bare LCO and TMA-LCO. a,b\ , Scanning electron microscopy \(SEM\) images of bare LCO \(a\) and TMA-LCO \(b\). Scale bars: 20 m. c, Cross-sectional TEM\ image of TMA-LCO. Scale bar: 2 m. :2541)/F 4/H/N/Rect[60.2142 55.2059 73.4015 42.6602]/Subtype/Link/Type/Annot>> endobj 6 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 2 | Electrochemical characterization of bare LCO and TMA-LCO. a, Comparis\ on of cycle performances of LiCoO2|Li half cells with bare LCO versus TMA-LCO. b,c, Charge discharge curves of bare LCO \(\ b\) and TMA-LCO \(c\) half cells :2542)/F 4/H/N/Rect[384.816 590.706 402.151 578.16]/Subtype/Link/Type/Annot>> endobj 7 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 2 | Electrochemical characterization of bare LCO and TMA-LCO. a, Compari\ son of cycle performances of LiCoO2|Li half cells with bare LCO versus TMA-LCO. b,c, Charge discharge curves of bare LCO \(\ b\) and TMA-LCO \(c\) half cells:2543)/F 4/H/N/Rect[511.685 443.706 526.658 431.16]/Subtype/Link/Type/Annot>> endobj 8 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 2 | Electrochemical characterization of bare LCO and TMA-LCO. a, Compar\ ison of cycle performances of LiCoO2|Li half cells with bare LCO versus TMA-LCO. b,c, Charge discharge curves of bare LCO \ \(b\) and TMA-LCO \(c\) half cell:2544)/F 4/H/N/Rect[374.073 317.706 383.391 305.16]/Subtype/Link/Type/Annot>> endobj 9 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 2 | Electrochemical characterization of bare LCO and TMA-LCO. a, Compa\ rison of cycle performances of LiCoO2|Li half cells with bare LCO versus TMA-LCO. b,c, Charge discharge curves of bare LCO\ \(b\) and TMA-LCO \(c\) half cel:2545)/F 4/H/N/Rect[483.65 212.706 492.01 200.16]/Subtype/Link/Type/Annot>> endobj 10 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 3 | Structural evolution during the initial charge discharge process. a,\ b, Insitu XRD evolution of bare LCO \(a\) and TMA-LCO \(b\) at the \(003\) and \(107\) diffraction peaks, with the correspondi\ ng charge discharge curves aligned to:2546)/F 4/H/N/Rect[481.976 76.2059 497.097 63.6602]/Subtype/Link/Type/Annot>> endobj 11 0 obj <>/BS<>/Border[0 0 0]/F 4/H/N/Rect[464.865 33.864 552.756 25.1497]/Subtype/Link/Type/Annot>> endobj 12 0 obj <>/ExtGState<>/Font<>/ProcSet[/PDF/Text]/XObject<>>> endobj 13 0 obj <>stream x][oFv~C2PsXsX`23lNlfQ:ZZh2<$ԩ˩ ؈ RIV:\o-ٳnٿٳxV$qs_.\;[EQ%φ*R~Vy#vDҕ}={:e&Y'=3QU31OmKvw AJ?d}WM+r!^;xL<DzHqilU pEMoLT]֥7;s>MЦ*FmP']eyf.uEg{z*V|V@d6&Z .P`JfG(p`>%>)B~ܦwt[6j<#@SfO+y l쾿!-k7Yd\s@*!NROXR0""v&voMj[yTkBM]p!m$tT+S 0w@jb& luwAj~rRɋT\`J8|(O.$iL<%VDv; %j_˯6y] N/U5p)\}%:: ̔Rꊼܡʲ iEᣐݨ7EurљIc7I\Y|7qLlJaW#PQ ʙmϞP|UH|D)j[sХR'?*,}P;_"ǽ>0=4]V4Q <:(˹mIDAVULܲBfVsIiN]oO_)\}CPb,/n۽UV+Z3k+dAEin V\U8x^D [Hee5noiラZa(ď6D{Y`uvE=c0ڸpm%$ˊ%Z1$`UPo*kU @%0Aa$0YslB G1R.ctnk)BXl#7Ue%\,vNRuˌdDLA**ܚ%@(-:KOs.9/H0I`*& ]O>=&ag$E[&mQ:iPzN2ȅ\ͳoׇ_or>勳4gzK (1eX\!b\oc!=D<.GVSK#tC' 6I/!>$J XI+"iwYgHHjiWp;%H:oyS(c&+>'b(kE ˇ>ptgX B t"rh \)Kfo;'A<:@$0q퉲?'-: 9,f#- WXFAϓudjEX$MY~iZ/r]; ȝF] 9)b!D73 `ʹ9gO+Ը=Scmd"Vik8. 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Vander Ven, A., Aydinol, M. K., Ceder, G., Kresse, G. & Hafner, J. First-princ\ iples investigation of phase stability in LixCoO2. Phys. Rev. B 58, 2975 2987 \(1998\).\r:2548)/F 4/H/N/Rect[74.554 296.706 79.7589 284.16]/Subtype/Link/Type/Annot>> endobj 20 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd: 29. Amatucci, G. G., Tarascon, J. M. & Klein, L. C. CoO2, the end member of the L\ ixCoO2 solid solution. J. Electrochem. Soc. 143, 1114 1123 \(1996\).\r:2549)/F 4/H/N/Rect[80.9951 296.706 86.2 284.16]/Subtype/Link/Type/Annot>> endobj 21 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 3 | Structural evolution during the initial charge discharge process. a\ ,b, Insitu XRD evolution of bare LCO \(a\) and TMA-LCO \(b\) at the \(003\) and \(107\) diffraction peaks, with the correspon\ ding charge discharge curves aligned :2550)/F 4/H/N/Rect[58.6287 275.706 73.7504 263.16]/Subtype/Link/Type/Annot>> endobj 22 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd: 30. Reimers, J. N. & Dahn, J. R. Electrochemical and insitu X-ray diffraction stud\ ies of lithium intercalation in LixCoO2. J. Electrochem. Soc. 139, 2091 2097 \(1992\).\r:2551)/F 4/H/N/Rect[63.407 254.706 68.612 242.16]/Subtype/Link/Type/Annot>> endobj 23 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd: 31. Yang, S.-H., Levasseur, S., Weill, F. & Delmas, C. Probing lithium and vacancy \ ordering in O3 layered LixCoO2 \(x "H 0.5\): an electron diffraction study. J. Electrochem. Soc. 150, A366 A373 \(2003\).\ \r:2552)/F 4/H/N/Rect[69.8482 254.706 75.0531 242.16]/Subtype/Link/Type/Annot>> endobj 24 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 3 | Structural evolution during the initial charge discharge process. a\ ,b, Insitu XRD evolution of bare LCO \(a\) and TMA-LCO \(b\) at the \(003\) and \(107\) diffraction peaks, with the correspo\ nding charge discharge curves aligned:2553)/F 4/H/N/Rect[236.526 202.206 244.924 189.66]/Subtype/Link/Type/Annot>> endobj 25 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO. \ a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmission X-r\ ay microscopy. Scale bar: 1 m. d :2554)/F 4/H/N/Rect[332.475 328.206 349.791 315.66]/Subtype/Link/Type/Annot>> endobj 26 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO. \ a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmission X-\ ray microscopy. Scale bar: 1 m. d:2555)/F 4/H/N/Rect[383.241 328.206 400.204 315.66]/Subtype/Link/Type/Annot>> endobj 27 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO.\ a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmission X\ -ray microscopy. Scale bar: 1 m. d:2556)/F 4/H/N/Rect[343.513 286.206 359.091 273.66]/Subtype/Link/Type/Annot>> endobj 28 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO.\ a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmission \ X-ray microscopy. Scale bar: 1 m. :2557)/F 4/H/N/Rect[486.759 265.206 500.03 252.66]/Subtype/Link/Type/Annot>> endobj 29 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO.\ a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmission\ X-ray microscopy. Scale bar: 1 m. :2558)/F 4/H/N/Rect[539.476 244.206 547.418 231.66]/Subtype/Link/Type/Annot>> endobj 30 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LCO\ . a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmissio\ n X-ray microscopy. Scale bar: 1 m.:2559)/F 4/H/N/Rect[500.551 191.706 509.395 179.16]/Subtype/Link/Type/Annot>> endobj 31 0 obj <>/BS<>/Border[0 0 0]/Dest(SpringerNature_NatEner_409.indd:Fig. 4 | 3D X-ray tomography reconstruction and element distribution in TMA-LC\ O. a c, 3D spatial distributions of Al \(a\), Co \(b\) and Ti \(c\), probed by fluorescence-yield scanning transmissi\ on X-ray microscopy. 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